Because the output pulse from a Geiger–Müller tube is always of the same magnitude (regardless of the energy of the incident radiation), the tube cannot differentiate between radiation types.
No "signature" detection possible with simple counters I'm afraid.
They used trucks on the road with large doped sodium iodide crystal pack (tubes with a scintallation (flash) detector at the ends) that produce a second by second full spectrum of gamm energies seen.
Processing software is used to filter out cosmic radiation signatures, the ground vehicle signatures, the mean expected background signature of the Western Australian region, and to enhance the target peaks from the Cs-137 source.
You'd think that was quick, ... but generally this kind of thing would be done from a crop duster airframe flying at an industry standard 70m/sec (252 km/hr).
I'm guessing the local Perth geophysical survey companies that routinely fly magnetics and radiometrics were all fully engaged flying pre booked contract work .. so they dragged in a couple of white transit vans and fitted them out to get the job done.
Seems straightforward enough in the geophysical instrumentation domain.
Exotic? Radiometric mapping has been around for 50+ years - Australia has mapped the entire country (size of mainland contiguous USofA) from aircraft with ~200m line spacing in that time (along with surveying other countries, Mali, Fiji, India|Pakistan border, elsewhere), Russia, South Africa, Finland, USofA also have radiometric survey teams.
It's handy for finding drums of radioactive waste in a Finnish forrest near the Russia border, for example, which was an actual contest | exercise some years ago.
Australian civilian radiation services with backing of AGSO (Australian Geological Survey Organisation) are easily able to handle this all within Australia w/out reaching out to the Indians, Pakistani's, Iranians, Russians, South Africans, or other international nuclear agencies.
They used trucks on the road with large doped sodium iodide crystal pack (tubes with a scintallation (flash) detector at the ends) that produce a second by second full spectrum of gamm energies seen.
Processing software is used to filter out cosmic radiation signatures, the ground vehicle signatures, the mean expected background signature of the Western Australian region, and to enhance the target peaks from the Cs-137 source.