I currently have three around the apartment attached to the network:
One running Seafile (https://www.seafile.com/en/home/) with an old laptop hard-drive connected via USB enclosure. It acts as my own Dropbox. I mainly store notes and photos on it and sync them to a few other devices for redundancy. It also has a Samba share with all of my music and has an open vpn server so I can connect to it from anywhere.
Another with a GPIO breakout and breadboard with an individually addressable LED light strip attached. I got the idea from this Adafruit tutorial (https://learn.adafruit.com/light-painting-with-raspberry-pi/...). I wrote a program in Python to make it softly glow between random colors and sync to any beats-per-minute.