I don't presume to be aware of all the implementation details, but in the abstract, is this not a pretty excellent use of tax payer money? To support universal access to research, data, and educational materials?
Yes, but as others have said, professional advancement typically depends on publishing in the expensive journals. And that's no accident, in that predatory for-profit publishers have targeted prestigious journals for acquisition. It's the same game that drug makers play with top-selling drugs.
Eventually, authors will migrate to the not-for-profit open access journals and platforms. But that will take time. Top-ranked PIs must lead the way, given that their reputations are well established, and they have tenure.