That's easy to add.
In BinaryKeyboard.ino, the SendVal function [1] uses keyboard.write to send the keys. You can see a list of special keys you can send at https://www.arduino.cc/en/Reference/KeyboardModifiers but you'll need to use keyboard.press to hold down two keys at once. See https://www.arduino.cc/en/Reference/KeyboardPress which even has some example code.
[1] https://github.com/Chris-Johnston/BinaryKeyboard/blob/master...